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Global Sensitivity Analysis of Tropospheric Ozone and OH: Budgets from three global chemistry-climate models

This dataset contains monthly mean global atmospheric distributions of ozone mixing ratio and methane chemical loss rate (the largest sink for atmospheric methane is the hydroxyl radical, OH) from 105 model runs with three independent global chemistry climate models. The models include the Frontier Research System for Global Change version of the University of California, Irvine Chemical Transport Model (FRSGC/UCI CTM), the Goddard Institute for Space Studies Global Climate Model (GISS GCM) and the Community Atmosphere Model with Chemistry (CAM-Chem). All three models performed the same simulations for a one-year period (broadly representative of 2001 meteorology) under standardised conditions (40 TgN/yr surface NOx emissions, 5 TgN/yr lightning emissions, 500 TgC/yr biogenic isoprene emissions, 1760 ppb tropospheric methane). An ensemble of 105 simulations was performed that included a control run (run 0), a set of runs that were used to build Gaussian Process emulators (runs 1-80), and additional runs that were used to evaluate the emulators (runs 81-104). A spin-up of six months was performed for each run, and monthly mean model results were archived for the following 12 months. The meteorological conditions used were the same in each simulation.



The data supports the exploration of the sensitivity of tropospheric ozone and the chemical lifetime of methane in the troposphere (a proxy for the hydroxyl radical, OH) to eight variables: (1) NOx emissions from all surface sources (range: 30-50 TgN/yr), (2) NO emissions from lightning (range: 2-8 TgN/yr), (3) biogenic isoprene emissions (range: 200-800 TgC/yr), (4) dry deposition rates of all deposited species (range: +/- 80%), (5) wet deposition rates of all soluble species (range: +/- 80%), (6) atmospheric humidity as used in the chemistry scheme only (range: +/- 50%), (7) cloud optical depth (range: factor of 10), and (8) turbulent mixing in the planetary boundary layer (range: factor of 100). The design of the ensemble runs used a Latin Hypercube method to sample this eight-dimensional parameter space to achieve optimal coverage with only 80 simulations. A separate design was used to select an additional 24 simulations to evaluate the emulators built from the standard 80 runs. The specifications for each simulation (total annual emission rate for surface NOx, biogenic isoprene and lightning NO, and the scaling factors applied to native model dry and wet deposition rates, humidity, cloud optical depth, and boundary layer diffusion coefficient) are provided with the dataset.

Simple

Date (Publication)
2020-04-24T09:55:52
Date (Creation)
2020-04-24T09:55:52
Citation identifier
https://catalogue.ceda.ac.uk/uuid/d5afa10e50b44229b079c7c5a036e660
Citation identifier
Centre for Environmental Data Analysis (CEDA) / d5afa10e50b44229b079c7c5a036e660
Point of contact
Organisation name Individual name Electronic mail address Role

Unavailable

Wild, Oliver

Unavailable

Author

Unavailable

Voulgarakis, Apostolos

Unavailable

Author

Unavailable

Lamarque, Jean-Francois

Unavailable

Author

Centre for Environmental Data Analysis (CEDA)

support@ceda.ac.uk

Custodian

Centre for Environmental Data Analysis (CEDA)

support@ceda.ac.uk

Distributor

Unavailable

Wild, Oliver

Unavailable

Principal investigator

Centre for Environmental Data Analysis (CEDA)

support@ceda.ac.uk

pointofContact

Unavailable

Wild, Oliver

Unavailable

pointofContact

Centre for Environmental Data Analysis (CEDA)

support@ceda.ac.uk

Publisher
Maintenance and update frequency
Not planned
Update scope
Dataset
Keywords
  • Tropospheric ozone burden

  • tropospheric methane lifetime

  • Gaussian process emulation

  • sensitivity analysis

GEMET - INSPIRE themes, version 1.0

  • atmospheric conditions

Access constraints
Other restrictions
Other constraints
Public data: access to these data is available to both registered and non-registered users.
Use constraints
Other restrictions
Other constraints
Under the following licence http://www.nationalarchives.gov.uk/doc/open-government-licence/version/3/, appropriate use of these data may fall under any use. This message is intended as guidance, always read the full licence. When using these data you must cite them correctly using the citation given on the CEDA Data Catalogue record.
Spatial representation type
Grid
Language
English
Topic category
  • Climatology, meteorology, atmosphere
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Begin date
2001-01-01T00:00:00
End date
2001-12-31T00:00:00
Unique resource identifier
WGS 84
Distribution format
Name Version

Data are netCDF formatted.

Distributor contact
Organisation name Individual name Electronic mail address Role

Centre for Environmental Data Analysis (CEDA)

support@ceda.ac.uk

Distributor
OnLine resource
Protocol Linkage Name
https://catalogue.ceda.ac.uk/uuid/d5afa10e50b44229b079c7c5a036e660

CEDA Data Catalogue Page

OnLine resource
Protocol Linkage Name
http://data.ceda.ac.uk/badc/deposited2020/QRU-TropO3OH/data

DOWNLOAD

OnLine resource
Protocol Linkage Name
https://www.atmos-chem-phys-discuss.net/acp-2019-774/

Global sensitivity analysis of chemistry-climate model budgets of tropospheric ozone and OH: Exploring model diversity

OnLine resource
Protocol Linkage Name
http://data.ceda.ac.uk/badc/deposited2020/QRU-TropO3OH/metadata/run_specifications.txt

Run specifications of used for the Global Sensitivity Analysis of Tropospheric Ozone and OH model runs

Hierarchy level
Dataset

Conformance result

Title

Commission Regulation (EU) No 1089/2010 of 23 November 2010 implementing Directive 2007/2/EC of the European Parliament and of the Council as regards interoperability of spatial data sets and services

Date (Publication)
2010-12-08
Statement

Original global model results generated for the NERC project "Quantifying and Reducing Uncertainty in the Processes Controlling Tropospheric Ozone and OH". Selected variables provided in NetCDF format by model investigators and harmonized in CF-compliant NetCDF for submission to CEDA.

Metadata

File identifier
d5afa10e50b44229b079c7c5a036e660 XML
Metadata language
English
Character set
UTF8
Hierarchy level
Dataset
Date stamp
2026-02-05T03:20:11
Metadata standard name
UK GEMINI
Metadata standard version

2.3

Metadata author
Organisation name Individual name Electronic mail address Role

Centre for Environmental Data Analysis (CEDA)

support@ceda.ac.uk

Point of contact
 
 

Overviews

Spatial extent

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Keywords

GEMET - INSPIRE themes, version 1.0

atmospheric conditions


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